Full Cast — Captain Scarlet and the Mysterons (1967–1968)
Francis Matthews
Captain Scarlet (voice)
Ed Bishop
Narrator / Captain Blue (voice)
Donald Gray
The Mysterons / Colonel White / Captain Black (voice)
Cy Grant
Lieutenant Green (voice)
Jeremy Wilkin
Morton / Distillery Attendant (voice) / Jackson (voice) / Dr. Denton / Spectrum, New York (voice) / Human Captain Black / Delta Garage Attendant / Radio Announcer (voice) / Captain Ochre / Barman (voice) / Colonel Storm / Robot (voice) / Rhodes (voice) / Kinley (voice) / Andre Verdain +37 more
Gary Files
Captain Magenta / Pilot (voice) / Engineer / Security Guard (voice) / Cadet Phil Machin (voice) / Neilson (voice) / Sergeant (voice) / Photographer Joe / Flight Desk (voice) / Conrad Olafson (voice) / Captain Indigo / 1st Warden (Post 14) / 3rd Warden (Post 40) (voice) / Captain Magenta +24 more
Martin King
Richards / Garage Mechanic / Security Chief (voice) / DT19 Co-Pilot (voice) / Red Dear Sentry (Joe) / Cariboo Sentry (voice) / Vice President (voice) / Oil Worker (voice) / Dr. Theodore Magnus (voice) / Navigator (voice) / Orson / Speech Intelligence Decoder (voice) +21 more
Elizabeth Morgan
Destiny Angel / Airport Tannoy (voice) / Destiny Angel / Harmony Angel (voice) / Destiny Angel / Rhapsody Angel (voice) / Nurse (voice) / Destiny Angel (voice) / Destiny Angel / Nurse (voice) / Destiny Angel / Rhapsody Angel / Harmony Angel (voice) / Rhapsody Angel +3 more
Charles Tingwell
Space General Paterson (voice) / Doctor Fawn / Morgan (voice) / Macy (voice) / Captain Brown / Lieutenant Dean / Helicopter A42 Pilot (voice) / Harris (voice) / Macey / 4th Policeman (voice) / Captain Hassel (voice) / Fairfield (voice) / Base Controller (voice) / Carter (voice) +8 more
David Healy
Geiger Operator / Guard Voice 2 (voice) / General Rebus (voice) / Major Stone (voice) / Major Moran (voice) / Jason Smith (voice) / President Roberts (voice) / Frazer (voice) / Lunar Controller (voice) / Dr. Mitchell (voice) / General Cope / Major Brooks (voice) +6 more
Paul Maxwell
Captain - USS Panther II (voice) / Captain Grey / DT19 Pilot (voice) / General Ward (voice) / Base Commander (voice) / Supreme Commander of Earth Forces (voice) / Captain Grey / Guard (voice) / 1st Policeman (voice) / Captain Grey / General Tiempo / Porter Benson (voice) +6 more
Sylvia Anderson
Vice President's Wife (voice) / Melody Angel (voice) / Receptionist (voice) / Linda Nolan (voice) / Gabrielle (voice) / Judith Chapman (voice)
Janna Hill
Symphony Angel (voice) / Intercontinental Airlines Tannoy (voice)
Neil McCallum
4th Policeman (voice) / Airport Controller (voice) / Raynor (voice) / Professor G.A. Carney / Security Centre Guard (voice) / 2nd Policeman (voice)
Shane Rimmer
Pilot (voice) / Sergeant (voice) / Mason (voice)
Lian-Shin Yang
Harmony Angel (voice)